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Radiation degrades nuclear waste-containing materials faster than expected

Minerals intended to entrap nuclear waste for hundreds of thousands of years may be susceptible to structural breakdown within 1,400 years, a team from the University of Cambridge and the Pacific Northwest National Laboratory reported today (Jan. 11) in the journal Nature.

The new study used nuclear magnetic resonance, or NMR, to show that the effects of radiation from plutonium incorporated into the mineral zircon rapidly degrades the mineral's crystal structure.

This could lead to swelling, loss of physical strength and possible cracking of the mineral as soon as 210 years, well before the radioactivity had decayed to safe levels, said lead author and Cambridge earth scientist Ian Farnan.

According to current thinking, highly radioactive substances could be rendered less mobile by combining them, before disposal, with glass or with a synthetic mineral at a very high temperature to form a crystal.

However, the crystal structure can only hold the radioactive elements for so long. Inside the crystal radioactive decay occurs, and tiny atomic fragments called alpha particles shoot away from the decaying nucleus, which recoils like a rifle, with both types repeatedly blasting the structure until it breaks down.

This may increase the likelihood for radioactive materials to leak, although co-author William J. Weber, a fellow at the Department of Energy national laboratory in Richland, Wash., who made the samples used in the study, cautioned that this work did not address leakage, and researchers detected no cracking. Weber noted that the "amorphous," or structurally degraded, natural radiation-containing zircon can remain intact for millions of years and is one of the most durable materials on earth.

Some earth and materials scientists believe it is possible to create a structure that rebuilds itself after these "alpha events" so that it can contain the radioactive elements for much longer. The tests developed
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Contact: Bill Cannon
cannon@pnl.gov
509-375-3732
DOE/Pacific Northwest National Laboratory
10-Jan-2007


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